CE10 - Industrie et usine du futur : Homme, organisation, technologies 2021

Adaptive composite materials with machine learning and 4D printing – REDeSIGN4D

Adaptive composite materials with machine learning and 4D printing

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Challenges and objectives

REDeSIGN4D explores new bio-inspired, programmable shape-changing structures with controlled environmental impact. They are produced from flax fibers, combined with the use of innovative 4D printing, functionalization, multi-physics numerical simulation, and machine learning processes. Inspired by biological models such as the pine cone, hygromorphic biocomposites (HBCs) break with the current paradigm, which consists of combating the hygroscopic properties of plant fibers rather than seeking to take advantage of them. They were first developed at IRDL. These are materials architected by 4D printing, both sensors and actuators that change shape via a humidity gradient. REDeSIGN4D will help overcome certain obstacles such as: 1) The lack of knowledge on the forces that can be generated during their hygrostimulation. 2) The relatively slow response. 3) The uncontrolled response. 4) The low diversity of movement. Thus, to overcome these obstacles, the project team is working on: 1) Mastering the relationships between the parameters of the 4D printing process and the generation of forces through the involvement of machine learning. 2) The relationship between bioinspired architecture and the temporal response of HBCs. 3) The formulation/modification of conductive plant fibers to control the water content by Joule effect. 4) The implication of geometric effects such as instabilities.

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An experimental protocol was developed to evaluate the swelling pressure of hygromorphic biocomposites (HBCs) during immersion in water. These are composed of flax yarns coated with polymer (PLA) and produced by 4D printing. The experimental analysis allows us to characterize the blocking forces, the maximum expansion and various expansions under stress. Inspired by wood architecture, different HBC configurations are defined using slicing parameters (layer height, distance between filaments, orientation, etc.). Tests carried out on a rheometer allow us to obtain the «force-stroke« behaviors and ultimately the energy density. Spruce wood samples are used for comparison. The printed HBCs have highlighted an energy density that exceeds that of the spruce samples and which depends on the induced mesostructure. To control the water content of HBCs, flax yarns were functionalized in two different ways using either polypyrrole (PPy) or polypyrrole with silver (PPy-Ag). Ppy-coated flax yarns showed more homogeneous conductivity than flax-PPy-Ag. A maximum temperature increase of +20°C and +18°C for flax-PPy and flax-PPy-Ag, respectively.

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Ismael, A.; Beaugrand, J.; Castro, M.; le Duigou, A.; Guessasma, S.; Villares, A. Characterization of conductive and thermoactivated flax yarns using in-situ polymerization of polypyrrole, In preparation.

Ismael, A.; Beaugrand, J.; Castro, M.; Guessasma, S.; Villares, A. Functionalization of flax fibers to develop electroresponsive hygromorph biocomposites; 6th International Conference on the Natural Fibers (ICNF), Funchal, Portugal, June 19-21, 2023.

Ismael, A.; Beaugrand, J.; Castro, M.; Guessasma, S.; Villares, A. Journée Jeunes Chercheurs (7th), Jun. 2024 (poster and 1min30 oral presentation).

Ledru, J.B.; Castro, M.; Guessasma, S.; Le Duigou, A. Structural actuation of 4D printed hygromorph biocomposites, European Conference on Composite Material, Nantes, 2024.

Submission summary

The development of the industry of the future is based on innovation vectors such as eco-design, digital engineering, artificial intelligence and new materials obtained through innovative processes. The synergies created by the interaction between these different technologies are poorly understood and represent a disruptive potential which is the base for REDeSIGN 4D.
As part of défi 8 «Domaines transversaux», axe 13 « Industrie et usine du futur : Homme, organisation, technologies», REDeSIGN 4D explores technological bricks to create new adaptive bio-inspired structures with a controlled environmental impact. They will be eco-designed and produced from renewable and local resources, combined with the use of innovative 4D printing, functionalization, multi-physical digital simulation and machine learning processes.
Labeled by the EMC2 cluster, we have chosen as a case study hygromorphic biocomposites made from flax fibers, targeting promising benefits in several industrial sectors in demand (building, defense, energy, etc.). A second innovative axis lies in the systematic Life Cycle Analysis (LCA) to assess the environmental impacts of the proposed innovations.
Inspired by functional biological structures such as the pine cone, hygromorphic biocomposites break with the current paradigm which consists in fighting against the hygroscopic properties of plant fibers such as flax rather than seeking to benefit from them. These are architectural materials, both sensors and actuators that change shape (actuation or morphing) autonomously in the presence of a humidity gradient. At the same time, the advent of 4D printing, an extension of 3D printing dedicated to stimulable materials, opens up a field of possibilities in terms of the architecture of hygromorphic biocomposites.
The state of the art highlights 4 obstacles that REDeSIGN 4D will remove: 1) the mastery of the relationships between the parameters of the 4D printing process, 2) the slowness of the stimulated response and 3) the controlled prescription of the movements of the hygromorphic biocomposites and finally 4) the predictability of their multi-scale and multi-physical behavior.
REDeSIGN 4D is divided into four operational Work-Packages (WP1-4) corresponding to the 4 scientific and technical obstacles to be removed. The scope of skills is covered by the three partner laboratories (IRDL, INRAe BIA and PIMM) while relying on the recruitment of 3 doctoral students and one post-doctoral fellow. The environmental issues will be assessed throughout the 48 months by setting up an LCA approach, transversal to the WP.
First, at the mesoscopic scale we will apply statistical learning methodologies such as neural network (machine learning) to understand the effect of the process on the morphing capacity of hygromorphic biocomposites (WP1 months 0-36). At the same time, REDeSIGN 4D will propose on a microscopic scale an original functionalization of flax fibers to make them electrically active, in order to generate functionalized biocomposites whose potential for hygromorphism will be greater while benefiting moreover from the control of morphing by Joule effect (WP2 months 0-36). Based on this knowledge, using parametric and topological optimization processes, REDeSIGN 4D will propose, at the mesoscopic scale, architectural configurations of an optimized hygromorphic biocoposite fold allowing optimal and amplified morphing (WP3 months 0-36).
The last stage (WP4 months 30-48) makes the link between the work carried out in WPs 1, 2 and 3, via the realization of a structure known as "proof of concept" allowing to amplify, by structural effects, the morphing proposed by the hygromorphic biocomposite previously functionalized. We are therefore here at the largest scale, assembling the scales of the previous WPs.

Project coordination

Antoine Le Duigou (Institut de Recherche Dupuy de Lôme)

The author of this summary is the project coordinator, who is responsible for the content of this summary. The ANR declines any responsibility as for its contents.

Partnership

BIA Biopolymères, Interactions Assemblages
PIMM Procédés et Ingénierie en Mécanique et Matériaux
IRDL Institut de Recherche Dupuy de Lôme

Help of the ANR 522,973 euros
Beginning and duration of the scientific project: March 2022 - 48 Months

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