Acoustics for antiferromagnets – ACAF
This project focused on two different materials.
In the ferrimagnet GdCo, we are studying the AF dynamics triggered by SAWs at the angular compensation temperature, where magnetization will remain non-zero and detectable.
In FeRh AF, the challenge is to control the static AF state using SAWs, based on the magneto-structural nature of the AF-FM transition.
For both of these aspects, it is first necessary to grow the materials on a piezoelectric substrate in order to be able to electrically excite the surface acoustic waves, using an industrially proven method based on interdigitated combs.
The next step is to measure the acoustic transmission for these two systems as a function of temperature and magnetic field, as these two parameters can be used to adjust the resonance frequency of the magnetic modes. For the set of parameters that makes it coincide with the acoustic frequency, critical absorption is expected. The experimental setups developed in the laboratory provide access to a static and dynamic, temporal and spatial analysis of the phenomena involved in order to refine our understanding .
In FeRh, we understood how to dynamically modify the AF<>FM transition using surface acoustic waves.
We also characterized the strength of the magnetoelastic coupling, as well as the elastic constants, which are essential parameters for optimizing resonant structures.
Finally, in its purely ferromagnetic phase, we have also understood how to exploit magnetic memory—or hysteresis—to achieve resonance.
The project has also yielded a wealth of very interesting results on two topics not initially considered:
- Thermal modulation of the AF/FM fraction in this material. These results have led to a fruitful collaboration with a new team and constitute an important part of a student's thesis work.
- the magnetic hysteresis observed in ferromagnetic resonance experiments on metals.
Understanding and modeling the role of magnetic hysteresis in phonon-magnon interaction will ultimately improve the performance of magnetic field sensors based on surface wave devices. We have also contributed to a review article on this topic, to be published in 2025 in Journal Physics D (Marangolo et al).
The ACAF project is at the crossroads of two very exciting and promising fields that have emerged and gained increasing international visibility in recent years, namely antiferromagnets, for novel spintronic devices, and magneto-acoustics, for novel magnetization manipulation schemes. There is now a keen interest to use colinear antiferromagnets (AFMs) instead of ferromagnets (FM) to code information magnetically, e.g. on two orthogonal directions of the Néel vector. The immunity of AFMs to external magnetic fields because of their vanishing magnetization however makes it challenging to detect and control the antiferromagnetic (AF) state. To bypass the bottlenecks of static and dynamic manipulation of AFMs, the project will implement a well-known effect in an original fashion: strain waves in the hypersound range (acoustic waves) will be used to actuate on the AF dynamics via magnetoelasticity. More specifically we will use surface acoustic waves (SAWs). With their energy–efficient generation, low attenuation, and power-flow confined to the surface, they have proved over the last couple years to be a very relevant tool for non-inductive wave-manipulation of magnetization in ultra-thin ferromagnets, opening a new route toward “straintronics”. Via magneto-elasticity they generate an effective radio-frequency magnetic field, particularly efficient to actuate on magnetization dynamics when their frequency matches spin wave frequencies.
To investigate fundamentally the potential of SAWs to control AF states, we have chosen two magnetostrictive model systems that can function around room temperature in order to be compatible with potential applications. Both systems reintroduce a finite and variable magnetization that will ease the detection of its dynamics and/or the Néel vector manipulation. In GdCo, a ferrimagnet, we will assess the potential of SAWs to drive the dynamics at the temperature of angular momenta compensation, where the dynamics is AF-like but the magnetization does not cancel. In the AFM FeRh, the ambitious goal will be to control the static AF state using SAWs, relying on the first-order magneto-structural AFM-FM transition, very sensitive to strain. At constant temperature the SAW will induce a local transition to the FM state, allowing for magnetization rotation by 90 degrees, leaving the Néel vector rotated after returning to the AFM state.
The project will develop sample design and growth for efficient electrical generation of SAWs on thin optimized FeRh and GdCo layers and microstructures, magnetic and structural characterization of the samples, investigation of the magnon and phonon dispersions by Brillouin light scattering, optical time- and space domain observation of acoustically-driven AF dynamics and AF-FM transition. The project gathers three French laboratories with complementary skills and techniques, and benefits from a well-recognized expertise in magneto-acoustics. It also includes collaboration with two foreign laboratories, for FeRh growth and theory.
In the longer term, this project might open new routes to implement magnetic components with lower Joule dissipation as strain will be excited by electrical fields. It could also allow alternative data storage design in AF materials using the wave properties of SAWs: focusing, interferences, wave-front shaping and waveguiding, or remote accessing of bits thanks to the weak attenuation of SAWs.
Project coordination
Laura THEVENARD (Institut des nanosciences de Paris)
The author of this summary is the project coordinator, who is responsible for the content of this summary. The ANR declines any responsibility as for its contents.
Partnership
LPS Laboratoire de Physique des Solides
University of Mainz / SINOVA Group
INSP Institut des nanosciences de Paris
LSPM Laboratoire des Sciences des Procédés et des Matériaux
Brno University of Technology / CEITEC
Help of the ANR 498,112 euros
Beginning and duration of the scientific project:
- 48 Months